Time- and momentum-resolved probe of heat transport in photo-excited bismuth

Appl. Phys. Lett. 102, 181903 (2013).

J. Chen, M. Trigo, S. Fahy, É. D. Murray, Y. M. Sheu, T. Graber, R. Henning, Y. J. Chien, C. Uher , D. A. Reis.

 PULSE Institute, SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA and

Department of Photon Science and Applied Physics, Stanford University, Stanford, California 94305, USA and

Department of Physics, University College Cork, Cork, Ireland and

Department of Chemistry, University of California, Davis, California 95616, USA and

Center for Integrated Nanotechnologies, MS K771, Los Alamos National Laboratory, Los Alamos, New Mexico 87545, USA and

The Center for Advanced Radiation Sources, University of Chicago, Chicago, Illinois 60637, USA and

Department of Physics, University of Michigan, Ann Arbor, Michigan 48109-1040, USA.

 

Abstract

 

We use time- and momentum-resolved x-ray scattering to study thermalization in a photo-excited thin single crystal bismuth film on sapphire. The time-resolved changes of the diffusescattering show primarily a quasi-thermal phonon distribution that is established in ≲100psand that follows the time-scale of thermal transport. Ultrafast melting measurements under high laser excitation show that epitaxial regrowth of the liquid phase occurs on the time-scale of thermal transport across the bismuth-sapphire interface.

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